March 15, 2008
Journal Article

X-Ray Luminescence of LaF3:Tb3+ and LaF3:Ce3+, Tb3+ Water Soluble Nanoparticles

Abstract

Utilizing scintillation nanoparticles as agents for photodynamic therapy for cancer treatment necessitates the use of biocompatible and water soluble nanoparticles. In this article, we report the synthesis and X-ray luminescence of water soluble Ce and Tb doped LaF3 nanoparticles. The nanoparticles are conjugated with folic acid and meso-tetra (o-carboxyphenyl) porphyrin. X-ray luminescence is observed from the nanoparticles in both powder and solution samples. More importantly, singlet oxygen has been detected from the conjugated system following X-ray excitation. These preliminary observations indicate that water-soluble scintillation nanoparticles can be potentially used in photodynamic therapy for deep-tissue cancer treatment.

Revised: April 30, 2008 | Published: March 15, 2008

Citation

Liu Y., W. Chen, S. Wang, A.G. Joly, S.L. Westcott, and B.K. Woo. 2008. X-Ray Luminescence of LaF3:Tb3+ and LaF3:Ce3+, Tb3+ Water Soluble Nanoparticles. Journal of Applied Physics 103, no. 6:Art. No. 063105. PNNL-SA-56544. doi:10.1063/1.2890148