October 1, 2000
Journal Article

Structure and Vibrational Spectra of H+(H2O)8: Is the Excess Proton in a Symmetrical Hydrogen Bond?

Abstract

The energetics, structure, and vibrational spectra of a wide variety of H+(H2O)8 structures are calculated using density functional theory and second-order Møller–Plesset ab initio methods. In these isomers of H+(H2O)8 the local environment of the excess proton sometimes resembles a symmetric H5O2+ structure and sometimes H3O+, but many structures are intermediate between these two limits.

Revised: January 23, 2012 | Published: October 1, 2000

Citation

Ciobanu C.V., L. Ojamae, I. Shavitt, and S.J. Singer. 2000. Structure and Vibrational Spectra of H+(H2O)8: Is the Excess Proton in a Symmetrical Hydrogen Bond?. Journal of Chemical Physics 113, no. 13:5321-5330.