September 30, 2008
Report

Effect of Concrete Wasteform Properties on Radionuclide Migration

Abstract

The objective of this investigation was to initiate numerous sets of concrete-soil half-cell tests to quantify 1) diffusion of I and Tc from concrete into uncontaminated soil after 1 and 2 years, 2) I and Re (set 1) and Tc (set 2) diffusion from fractured concrete into uncontaminated soil, and 3) evaluate the moisture distribution profile within the sediment half-cell. These half-cells will be section in FY2009 and FY2010. Additionally, 1) concrete-soil half-cells initiated during FY2007 using fractured prepared with and without metallic iron, half of which were carbonated using carbonated, were sectioned to evaluate the diffusion of I and Re in the concrete part of the half-cell under unsaturated conditions (4%, 7%, and 15% by wt moisture content), 2) concrete-soil half cells containing Tc were sectioned to measure the diffusion profile in the soil half-cell unsaturated conditions (4%, 7%, and 15% by wt moisture content), and 3) solubility measurements of uranium solid phases were completed under concrete porewater conditions. The results of these tests are presented.

Revised: October 28, 2008 | Published: September 30, 2008

Citation

Wellman D.M., C.C. Bovaird, S.V. Mattigod, K.E. Parker, R.M. Ermi, and M.I. Wood. 2008. Effect of Concrete Wasteform Properties on Radionuclide Migration Richland, WA: Pacific Northwest National Laboratory.