April 30, 2007
Journal Article

Analysis of Percent On-Cell Reformation of Methane in SOFC Stacks and the Effects on Thermal, Electrical, and Mechanical Performance

Abstract

Numerical simulations were performed to determine the effect that varying the percent on-cell steam-methane reformation would have on the thermal, electrical, and mechanical performance of generic, planar solid oxide fuel cell stacks. The study was performed using three-dimensional model geometries for cross-, co-, and counter-flow configuration stacks of 10x10- and 20x20-cm cell sizes. The analysis predicted the stress and temperature difference would be minimized for the 10x10-cm counter- and cross-flow stacks when 40 to 50% of the reformation reaction occurred on the anode. Gross electrical power density was virtually unaffected by the reforming. The co-flow stack benefited most from the on-cell reforming and had the lowest anode stresses of the 20x20-cm stacks. The analyses also suggest that airflows associated with 15% air utilization may be required for cooling the larger (20x20-cm) stacks.

Revised: December 20, 2007 | Published: April 30, 2007

Citation

Recknagle K.P., B.J. Koeppel, X. Sun, M.A. Khaleel, S.T. Yokuda, and P. Singh. 2007. Analysis of Percent On-Cell Reformation of Methane in SOFC Stacks and the Effects on Thermal, Electrical, and Mechanical Performance. ECS Transactions 5, no. 1:473-480. PNNL-SA-53556.