PNNL

Abstract

The methods currently used by the International Atomic Energy Agency to account for nuclear materials at fuel fabrication facilities are time consuming and require in-field chemistry and operation by experts. Spectral X-ray radiography, along with advanced inverse algorithms, is an alternative inspection that could be completed noninvasively, without any in-field chemistry, with inspections of tens of seconds. The proposed inspection system and algorithms are presented here. The inverse algorithm uses total variation regularization and adaptive regularization parameter selection with the unbiased predictive risk estimator. Performance of the system is quantified with simulated X-ray inspection data and sensitivity of the output is tested against various inspection system instabilities. Material quantification from a fully-characterized inspection system is shown to be very accurate, with biases on nuclear material estimations of