March 15, 2008
Journal Article

Heterogeneous Reduction of Tc(VII) by Fe(II) at the Solid-Water Interface

Abstract

Technetium-99 is a byproduct of uranium fission. It exists in two stable valence states (IV/VII) and exhibits a half-cell potential of intermediate value (Eo = 0.748 V). The oxidized form of 99Tc [pertechnetate, TcO4-] is an oxyanion that sorbs poorly to amphoteric surfaces and forms few solid phases with geochemically relevant cations. It is consequently highly mobile in oxic water-rock systems. The reduced valence state [Tc(IV)] is relatively insoluble (

Revised: April 7, 2011 | Published: March 15, 2008

Citation

Peretyazhko T., J.M. Zachara, S.M. Heald, B. Jeon, R.K. Kukkadapu, C. Liu, and D.A. Moore, et al. 2008. Heterogeneous Reduction of Tc(VII) by Fe(II) at the Solid-Water Interface. Geochimica et Cosmochimica Acta 72, no. 6:1521-1539. PNNL-SA-56929. doi:10.1016/j.gca.2008.01.004