September 1, 2017
Report

Evaluation of Iodine Remediation Technologies in Subsurface Sediments: Interim Status Report

Abstract

Isotopes of iodine were generated during plutonium production from nine production reactors at the U.S. Department of Energy Hanford Site. The long half-life 129I generated at the Hanford Site during reactor operations was 1) stored in single-shell and double-shell tanks, 2) discharged to liquid disposal sites (e.g., cribs and trenches), 3) released to the atmosphere during fuel reprocessing operations, or 4) captured by off-gas absorbent devices (silver reactors) at chemical separations plants (PUREX, B-Plant, T-Plant, and REDOX). Releases of 129I to the subsurface have resulted in several large, though dilute, plumes in the groundwater, including the plume in the 200-UP-1 operable unit. There is also 129I remaining in the vadose zone beneath disposal or leak locations. Because 129I is an uncommon contaminant, relevant remediation experience and scientific literature are limited.

Revised: September 26, 2018 | Published: September 1, 2017

Citation

Strickland C.E., A.R. Lawter, N. Qafoku, J.E. Szecsody, M.J. Truex, and G. Wang. 2017. Evaluation of Iodine Remediation Technologies in Subsurface Sediments: Interim Status Report Richland, WA: Pacific Northwest National Laboratory. doi:10.2172/1418095.