Lithium ion and lithium metal batteries have received tremendous interest in the last decade for a wide range of energy storage applications. Although great progress has been made in developing new electrode materials and concepts, it is difficult to rapidly incorporate these advances in battery technologies. A key challenge is the knowledge gap between the fundamental materials research and the cell-level understanding of the relationship between high energy and stable cycling. As a result, the literature reports are based on a wide range of experimental conditions that cannot be easily realized in realistic cells. Taking lithium metal batteries as an example, this paper briefly discusses the fundamental mechanisms that lead to the inconsistent observations in battery research. We then propose development of a standard testing protocol based on the requirements of high-energy lithium metal cells. The importance of building a standard testing protocol is emphasized to accelerate the discovery of solutions for real challenges as well as inspire innovations that are readily adaptable to real batteries.
Revised: May 21, 2019 |
Published: April 17, 2019
Citation
Chen S., C. Niu, H. Lee, Q. Li, L. Yu, W. Xu, and J. Zhang, et al. 2019.Critical Parameters for Evaluating Coin Cells and Pouch Cells of Rechargeable Li-Metal Batteries.Joule 3, no. 4:1094-1105.PNNL-SA-131547.doi:10.1016/j.joule.2019.02.004