April 10, 2019
Journal Article

A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water

Abstract

We present the laboratory results of immersion freezing efficiencies of cellulose particles at supercooled temperature (T) conditions. Three types of chemically homogeneous cellulose samples are used as surrogates that represent supermicron and submicron ice nucleating plant structural polymers. These samples include micro-crystalline cellulose (MCC), fibrous cellulose (FC) and nano-crystalline cellulose (NCC). Our experimental data show that particles resembling the MCC lab particle occur also in the atmosphere. Our immersion freezing dataset includes data from various ice nucleation measurement techniques available at seventeen different institutions, including nine dry dispersion and eleven aqueous suspension techniques. With a total of twenty methods, we performed systematic accuracy and precision analysis of measurements from all twenty measurement techniques by evaluating T-binned (1 °C) data over a wide T range (-36 °C

Revised: June 4, 2019 | Published: April 10, 2019

Citation

Hiranuma N., K. Adachi, D.M. Bell, F. Belosi, H. Beydoun, B. Bhaduri, and H. Bingemer, et al. 2019. A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water. Atmospheric Chemistry and Physics 19, no. 7:4823-4849. PNNL-SA-141665. doi:10.5194/acp-19-4823-2019