February 21, 2012
Journal Article

Large Amplitude Spatial and Temporal Gradients in Atmospheric Boundary Layer CO2 Mole Fractions Detected With a Tower-Based Network in the U.S. Upper Midwest

Abstract

This study presents observations of atmospheric CO2 mole fraction from a nine-tower, regional network deployed during the North American Carbon Program’s Mid-Continent Intensive during 2007 2009. Within this network in a largely agricultural area, mean atmospheric CO2 gradients were strongly correlated with both ground-based inventory data and estimates from satellite remote sensing. The average seasonal drawdown for corn-dominated sites (35 ppm) is significantly larger than has been observed at other continental boundary layer sites. Observed growing-season median CO2 gradients are strongly dependent on local flux. The gradients between cross-vegetation site-pairs, for example, average 2.0 ppm/100 km, four times larger than the similar-vegetation site-pair average. Daily-timescale gradients are as large as 5.5 ppm/100 km, but dominated by advection rather than local flux. Flooding in 2008 led to a region-wide 23 week delay in growing-season minima. The observations show that regional-scale CO2 mole fraction networks yield large, coherent signals governed largely by regional sources and sinks of CO2

Revised: March 1, 2012 | Published: February 21, 2012

Citation

Miles N., S.J. Richardson, K.J. Davis, T. Lauvaux, A. Andrews, T.O. West, and V. Bandaru, et al. 2012. Large Amplitude Spatial and Temporal Gradients in Atmospheric Boundary Layer CO2 Mole Fractions Detected With a Tower-Based Network in the U.S. Upper Midwest. Journal of Geophysical Research: Biogeosciences 117. PNNL-SA-84752. doi:10.1029/2011JG001781