An online monitor has been designed, built, and tested that is capable of measuring the residual transuranic concentrations in processed high-level wastes with a detection limit of 370 Bq/ml (10 nCi/ml) in less than six hours. The monitor measures the (?,n) neutrons in the presence of gamma-ray fields up to 1 Sv/h (100 R/h). The optimum design was determined by Monte Carlo modeling and then tempered with practical engineering and cost considerations. A multiplicity counter is used in data acquisition to reject the large fraction of coincident and highly variable cosmic-ray-engendered background events and results in a S/N ratio ~1.
Revised: June 14, 2005 |
Published: February 1, 2005
Citation
Brodzinski R.L., R.A. Craig, S.D. Fink, W.K. Hensley, N. Holt, M.A. Knopf, and E.A. Lepel, et al. 2005.An Instrument for Measuring the TRU Concentration in High-Level Liquid Waste.Journal of Radioanalytical and Nuclear Chemistry 263, no. 3:625-628.PNNL-SA-43323.