June 6, 2012
Report

Initial proof-of-principle for near room temperature Xe and Kr separation from air with MOFs

Abstract

Materials were developed and tested in support of the U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Technology Separations and Waste Forms Campaign. Specifically, materials are being developed for the removal of Xenon and krypton from gaseous products of nuclear fuel reprocessing unit operations. During FY 2012, Three Metal organic framework (MOF) structures were investigated in greater detail for the removal and storage of Xe and Kr from air at room temperature. Our breakthrough measurements on Nickel based MOF could capture and separate parts per million levels of Xe from Air (40 ppm Kr, 78% N2, 21% O2, 0.9% Ar, 0.03% CO2). Similarly, the selectivity can be changed from Xe > Kr to Xe

Revised: February 28, 2014 | Published: June 6, 2012

Citation

Thallapally P.K., and D.M. Strachan. 2012. Initial proof-of-principle for near room temperature Xe and Kr separation from air with MOFs Richland, WA: Pacific Northwest National Laboratory.